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ISDF

ISDF stands for interpolative separable density fitting, a numerical technique used in quantum chemistry to approximate electron repulsion integrals (ERIs). The method seeks a low-rank, separable representation of the four-index ERI tensor by introducing a small set of interpolation points and associated interpolation vectors. In practice, products of basis functions are approximated using information evaluated at these points, allowing the ERIs to be expressed as a sum over a modest number of auxiliary terms. This reduces both memory requirements and computational cost compared with conventional density fitting schemes, enabling more efficient HF, DFT, and post-HF calculations for larger systems or higher-accuracy treatments.

ISDF yields near-linear scaling with system size under common implementations and complements other acceleration techniques such

See also: density fitting, RI, tensor hypercontraction.

as
resolution-of-the-identity
(RI)
and
tensor
hypercontraction.
Limitations
include
the
nontrivial
selection
of
interpolation
points,
potential
loss
of
accuracy
if
the
point
set
is
insufficient,
and
added
algorithmic
complexity
in
some
software
pipelines.
ISDF
variants
include
randomized
sampling
procedures
to
choose
interpolation
points
and
adaptive
schemes
that
adjust
the
auxiliary
set
in
response
to
target
accuracy.